期刊
ACS NANO
卷 13, 期 11, 页码 12385-12392出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.9b05088
关键词
2D materials; MXenes; liquid-liquid interfaces; self-assembly; structured liquids
类别
资金
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division within the Adaptive Interfacial Assemblies Towards Structuring Liquids Program [DE-AC02-05-CH11231, KCTR16]
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under sp2Bonded Materials Program [DE-AC02-05-CH11231, KC2207]
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0018618]
The self-assembly of nanoscale materials at the liquid liquid interface allows for fabrication of threedimensionally structured liquids with nearly arbitrary geometries and tailored electronic, optical, and magnetic properties. Two-dimensional (2D) materials are highly anisotropic, with thicknesses on the order of a nanometer and lateral dimensions upward of hundreds of nanometers to micrometers. Controlling the assembly of these materials has direct implications for their properties and performance. We here describe the interfacial assembly and jamming of Ti3C2Tx MXene nanosheets at the oil water interface. Planar, as well as complex, programmed three-dimensional all-liquid objects are realized. Our approach presents potential for the creation of all-liquid 3D-printed devices for possible applications in all-liquid electrochemical and energy storage devices and electrically active, all-liquid fluidics that exploits the versatile structure, functionality, and reconfigurability of liquids.
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