期刊
SCRIPTA MATERIALIA
卷 170, 期 -, 页码 166-171出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.scriptamat.2019.05.034
关键词
Dielectric response; Sintering atmosphere; Giant permittivity; SrTiO3 ceramics
类别
资金
- NSFC-Guangdong Joint Funds of the Natural Science Foundation of China [W601209]
- National Key Basic Research Program of China (973 Program) [2015CB654601]
- Technical Innovation Special Program of Hubei Province [2017AHB055]
- Open Project of Key Laboratory of New Electric Functional Materials of Guangxi Colleges and Universities [DGN201505]
- State Key Laboratory of Advanced Technology Materials Synthesis and Processing (Wuhan University of Technology) [2018-KF-11]
- Natural Science Foundation of China [51872213]
Effects of sintering and annealing atmosphere on the defect structures and the dielectric behaviors of (Nb + Zn) co-doped SrTiO3 ceramics are systematically investigated. Giant permittivity (-50,100), low dielectric loss (similar to 0.04) and wide temperature (25-330 degrees C)/frequency (20-10(5) Hz) stabilities are achieved in the N-2 sintering ceramics. Further investigations indicate massive defects and defect clusters are involved, contributing to the giant permittivity. The associated defects not only restrain the ionization of oxygen vacancy, but also localize the motions of oxygen vacancy and electron, resulting in the low dielectric loss and the suppressed relaxation peaks. (C) 2019 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
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