4.8 Article

Polaron Mobility in the Beyond Quasiparticles Regime

期刊

PHYSICAL REVIEW LETTERS
卷 123, 期 7, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.123.076601

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资金

  1. National Science Foundation [PHY-1607611, DMR-1720465, DMR-1720816]
  2. Simons Collaboration on the Many Electron Problem
  3. ImPACT Program of the Council for Science, Technology and Innovation (Cabinet Office, Government of Japan), Japan [JPMJCR1874]
  4. JST CREST, Japan [JPMJCR1874]
  5. FP7/ERC Consolidator Grant QSIMCORR [771891]
  6. Nanosystems Initiative Munich
  7. Munich Center for Quantum Science and Technology

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In a number of physical situations, frompolarons to Dirac liquids and to non-Fermi liquids, one encounters the beyond quasiparticles regime, in which the inelastic scattering rate exceeds the thermal energy of quasiparticles. Transport in this regime cannot be described by the kinetic equation. We employ the diagrammatic Monte Carlo method to study the mobility of a Frohlich polaron in this regime and discover a number of nonperturbative effects: a strong violation of the Mott-Ioffe-Regel criterion at intermediate and strong couplings, a mobility minimum at T similar to Omega in the strong-coupling limit (Omega is the optical mode frequency), a substantial delay in the onset of an exponential dependence of the mobility for T < Omega at intermediate coupling, and complete smearing of the Drude peak at strong coupling. These effects should be taken into account when interpreting mobility data in materials with strong electron-phonon coupling.

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