期刊
ORGANIC LETTERS
卷 21, 期 16, 页码 6295-6299出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b02172
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资金
- Australian Research Council
- ANU Institute of Advanced Studies
- National Natural Science Fund of China [81872759]
- Pearl River Scholar Program of Guangdong Province
Synthetically derived (Z)-ligustilide (1) has been subjected to photochemically-promoted dimerization processes under a range of conditions. By such means, varying distributions of the dimeric natural products tokinolides A-C (4, 3, and 6, respectively) and riligustilide (5) as well certain related (isomeric) compounds have been obtained. The structures of three of them have been confirmed by single-crystal X-ray analysis. The biosynthetic implications of the outcomes of this study are discussed.
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