Broadband and narrowband laser-based terahertz source and its application for resonant and non-resonant excitation of antiferromagnetic modes in NiO

A versatile table-top high-intense source of terahertz radiation, enabling to generate pulses of both broadband and narrowband spectra with a tunable frequency up to 3 THz is presented. The terahertz radiation pulses are generated by optical rectification of femtosecond pulses of Cr:forsterite laser setup in nonlinear organic crystal OH1. Electric field strengths of broadband and narrowband terahertz pulses were achieved close to 20 MV/cm and more than 2 MV/cm, correspondingly. Experiments on excitation of spin subsystem oscillations of an anti ferromagnetic NiO were carried out. Selective excitation of 0.42 THz mode was observed for the first time at room temperature by a narrowband terahertz pulses tuned close to mode frequency. (C) 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement