期刊
NANO LETTERS
卷 19, 期 9, 页码 6511-6516出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.9b02740
关键词
Nonlinear holography; 2D materials; transition metal dichalcogenide monolayer; second-harmonic generation
类别
资金
- Office of Naval Research [N00014-16-1-2408]
- National Science Foundation [ECCS-1653032, DMR-1552871]
Nonlinear holography enables optical beam generation and holographic image reconstruction at new frequencies other than the excitation fundamental frequency, providing pathways toward unprecedented applications in optical information processing and data security. So far, plasmonic metasurfaces with the thickness of tens of nanometers have been mostly adopted for realizing nonlinear holograms with the potential of on-chip integration but suffering from low conversion efficiency and high absorption loss. Here, we report a nonlinear transition metal dichalcogenide (TMD) hologram with high conversion efficiency and atomic thickness made of only single nanopatterned tungsten disulfide (WS2) monolayer, for producing optical vortex beams and Airy beams as well as reconstructing complex holographic images at the second harmonic (SH) frequency. Our concept of nonlinear TMD holograms paves the way toward not only the understanding of light-matter interactions at the atomic level but the integration of functional TMD-based devices with atomic thickness into the next-generation photonic circuits for optical communication, high-density optical data storage, and information security.
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