4.2 Article

CO2 hydrogenation on Fe-based catalysts doped with potassium in gas phase and under supercritical conditions

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MENDELEEV COMMUNICATIONS
卷 29, 期 4, 页码 382-384

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DOI: 10.1016/j.mencom.2019.07.007

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New catalysts FeK/Sibunit and FeCuK/Sibunit were prepared and applied for the CO2 hydrogenation in the temperature range of 250-400 degrees C and under the pressures of 1, 20 and 85 atm. The reverse water gas shift reaction prevailed under the atmospheric pressure (i.e., CO2 was selectively converted into CO), while the formation of C-1-C-12 hydrocarbons occurred under the increased pressures. The Cu-containing catalyst exhibited the higher activity and selectivity towards C-1-C-12 hydrocarbons.

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