期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 391, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2019.121147
关键词
Negative emission technology; Sustainable waste management; Engineered biochar; Sustainable Development Goals (SDGs); Waste recycling/valorization
资金
- Korea Ministry of Environment (MOE) [2018002490001]
- Hydrogen Energy Innovation Technology Development Program of the National Research Foundation of Korea (NRF) - Korean government (Ministry of Science and ICT(MSIT)) [NRF-2019M3E6A1064197]
- Korea Environmental Industry & Technology Institute (KEITI) [ARQ201804021003] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
- National Research Foundation of Korea [2019M3E6A1064020] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
Biochar is newly proposed as an innovative and cost-effective material to capture CO2. In this study, biochar was produced from feedstock mixtures of food waste and wood waste (i.e., 20%:80% WFW20, 30%:70% WFW30 and 40%:60% WFW40) by gasification. The two biochar adsorbents containing the highest percentage of food waste, i.e., WFW40-K and WFW40-KC, were activated by KOH and KOH + CO2, respectively. The biochar adsorbents were then tested for CO2 adsorption at room temperature of 25 degrees C by using a volumetric sorption analyzer. The WFW20 showed the highest CO2 adsorption capacity, while higher percentage of food waste in the feedstock was unfavorable for the CO2 adsorption. The presence of N and S on the biochar surface was the primary contributor to the high CO2 uptake on WFW20. The development of micropores by KOH activation significantly increased the CO2 adsorption on WFW40-K, but KOH + CO2 activation could not further increase the development of micropores and subsequent CO2 adsorption. Moreover, WFW40-K showed >99% recyclability during 10 consecutive adsorption-desorption cycles. The biochars derived from biowaste (food waste and wood waste) could be effective adsorbents for CO2 capture by providing green solution for food waste recycling.
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