Polycyclic aromatic hydrocarbon (PAHs) geographical distribution in China and their source, risk assessment analysis

In China, the huge amounts of energy consumption caused severe carcinogenic polycyclic aromatic hydrocarbon (PAHs) concentration in the soil and ambient air. This paper summarized that the references published in 2008-2018 and suggested that biomass, coal and vehicular emissions were categorized as major sources of PAHs in China. In 2016, the emitted PAHs in China due to the incomplete combustion of fuel was about 32720 tonnes, and the contribution of the emission sources was the sequence: biomass combustion > residential coal combustion > vehicle > coke production > refine oil > power plant > natural gas combustion. The total amount of PAHs emission in China at 2016 was significantly decreased due to the decrease of the proportion of crop resides burning (indoor and open burning). The geographical distribution of PAHs concentration demonstrated that PAHs concentration in the urban soil is 0.092-4.733 mu g/g. At 2008-2012, the serious PAHs concentration in the urban soil occurred in the eastern China, which was shifted to western China after 2012. The concentration of particulate and gaseous PAHs in China is 1-151 ng/m3 and 1.08-217 ng/m3, respectively. The concentration of particle-bound PAHs in the southwest and eastern region are lower than that in north and central region of China. The incremental lifetime cancer risk (ILCR) analysis demonstrates that ILCR in the soil and ambient air in China is below the acceptable cancer risk level of 10-6 recommended by US Environmental Protection Agency (EPA), which mean that there is a low potential PAHs carcinogenic risk for the soil and ambient air in China. (C) 2019 Elsevier Ltd. All rights reserved.