期刊
COLLOIDS AND SURFACES B-BIOINTERFACES
卷 181, 期 -, 页码 226-233出版社
ELSEVIER
DOI: 10.1016/j.colsurfb.2019.05.048
关键词
Magnetic nanoparticles; Polydopamine; Fenton-like catalyst; Methylene blue; Removal
资金
- National Natural Science Foundation of China [51573078]
Fenton technology has been proven an effective way to remove dyes from wastewater. However, the demanding pH of reaction condition restricted its wide application. In this study, we report a novel Fenton-like catalyst (Fe3O4@PDA-MnO2) facilely synthesized by polydopamine (PDA) coating and MnO2 depositing onto the surface of Fe3O4 nanoparticles. This method for preparing magnetic Fe3O4@PDA-MnO2 catalyst could avoid the agglomeration of MnO2 nanoparticles and make the catalyst collect easily from the solution. The resultant Fe3O4@PDA-MnO2 nanoparticles possess core-shell nanostructure. Fe3O4@PDA-MnO2 catalyst could cooperate with hydrogen peroxide to form a Fenton-like reagent for the removal of methylene blue (MB) and performed excellent catalytic activities towards MB, including high degradation efficiency of 97.36% after 240 min. Besides, Fe3O4@PDA-MnO2 can retain excellent reusability after 5 using-cycles. More importantly, the catalyst can be used in a wide pH range from 2 to 12 in Fenton systems, demonstrating that the degradation process is independent on pH which is different from most reported studies. Also, Fe3O4@PDA-MnO2 could still keep more than 75% removal efficiency of MB in industrial wastewater treatment application. Therefore, the synthesized Fe3O4@PDA-MnO2 would be a promising device for the removal of dyes from wastewater.
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