期刊
CHEMICAL ENGINEERING JOURNAL
卷 372, 期 -, 页码 774-784出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2019.04.187
关键词
AOPs; Fe-0; Graphitized carbon; Sulfate radicals; Water remediation
资金
- National Natural Science Foundation of China [51878352, 51478224]
- priority academic program development of Jiangsu higher education institutions
The rational design of active and sustainable heterogeneous catalysts towards advanced oxidation process (AOPs) is of great significance for water remediation. Here, we synthesized Fe-0/graphitized carbon composite catalysts for efficient removal of bisphenol A (BPA) by activating peroxymonosulfate (PMS). The Fe-0/graphitized carbon composites were obtained by the pyrolysis of iron-tannic modified cotton, where tannic acid (TA) is an eco-friendly and low-cost polyphenol that can strongly form complexes with iron ions. The introduction of iron could significantly regulate the graphitization of carbon by changing the pyrolysis temperature. The combination of Fe-0 and graphitized carbon can endow Fe-TCs with an enhanced adsorption ability due to strong complexation between Fe-0 and BPA. The pyrolysis of iron-tannic modified cotton may serve as a novel strategy to design an efficient low-toxic metal-carbon catalyst for sulfate radical based processes in water remediation.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据