期刊
APPLIED SURFACE SCIENCE
卷 484, 期 -, 页码 1111-1117出版社
ELSEVIER
DOI: 10.1016/j.apsusc.2019.04.174
关键词
Co3S4/MoS2 nanocube; Prussian-blue analog; (NH4)(2)MoS4; Electrocatalytic property; Counter electrode; Dye-sensitized solar cell
类别
资金
- National Natural Science Foundation of China [21702031]
- Natural Science Foundation of Fujian Province [2018J01692]
- Hong Kong Scholars Program [XJ2018023]
Among clean energy catalysts, nanocube-structured functional materials with complex exterior texture, whose components/morphologies can be easily regulated, have attracted much attention. Hereon, we report the morphology-controllable Co3S4/MoS2 co-doped nanocubes (Co3S4/MoS2 NCs) derived from cobaltic Prussian-blue analog (Co PBA). The synthetic process of these nanocubes could be controlled by the reactant ratios (1/1, 1/2 and 1/3) of Co PBA to (NH4)(2)MoS4. In this process, (NH4)(2)MoS4 acted as a multifunctional vulcanizator, which could conveniently afford Mo and S elements at the same time. As the increment of (NH4)(2)MoS4, the exterior texture of Co3S4/MoS2 NCs became rougher with more embedded tiny nanoparticles. When the ratio was set as 1/2, the as-obtained Co3S4/MoS2-2 nanocubes exhibited good catalytic property in dye-sensitized solar cells (DSSCs). Notably, the DSSC with Co3S4/MoS2-2 counter electrode (CE) showed a better efficiency of 8.96% than that of Pt CE (7.77%) under standard conditions.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据