期刊
APPLIED CATALYSIS A-GENERAL
卷 586, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.apcata.2019.117214
关键词
Metal-organic frameworks; Heterogeneous catalysis; Single site
资金
- Inorganometallic Catalyst Design Center, an EFRC - DOE, Office of Science, Basic Energy Sciences [DE-SC0012702]
- Northwestern University Institute for Catalysis in Energy Processes (ICEP) - DOE, Office of Basic Energy Sciences [DE-FG02-03ER15457]
- Northwestern University
- NSF Graduate Research Fellowship [DGE-1842165]
Heterogeneous catalysts streamline industrial processes due to high stability and ease of separation. Efforts toward predictive catalytic activity and rational design of next-generation systems are impeded by structural ambiguity stemming from the presence of multiple irregular active sites within a catalyst. The uniformity of metal-organic frameworks (MOFs) provides a platform on which to develop single site catalysts in order to delineate atomically precise design rules. In this critical review, we highlight the development and progress of MOF-based single site catalysts and provide an outlook for further advancement of the field.
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