期刊
ADVANCED SCIENCE
卷 6, 期 17, 页码 -出版社
WILEY
DOI: 10.1002/advs.201900576
关键词
hierarchical; hollow; microtubes; oxyphosphides; water splitting
资金
- Ministry of Education of Singapore through AcRF Tier 2 grant [MOE2017-T2-2-003(S), M4020386]
- National Research Foundation (NRF) of Singapore via the NRF Investigatorship [NRF-NRFI2016-04]
Development of efficient electrocatalysts is a crucial requirement to build water splitting systems for the production of clean and sustainable fuels. This goal could be achieved by fine-tuning the composition and structure of the electrocatalytic materials. Here, a facile self-templated synthetic strategy is developed for the fabrication of hierarchical Co-Fe oxyphosphide microtubes (MTs). Fe-based metal-organic compound microrods are first synthesized as the self-sacrificing template. Afterward, the Fe-based precursors are converted into hierarchical Co-Fe layered double hydroxide MTs through a hydrothermal approach, which are then transformed into the hierarchical Co-Fe oxyphosphide MTs by a phosphidation treatment. Benefiting from the synergistic effect of the compositions and the advantages of the hierarchical hollow structure, the obtained electrocatalyst exhibits enhanced performance for overall water splitting.
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