期刊
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷 7, 期 16, 页码 13786-13795出版社
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.9b01559
关键词
Magnetic silica microrods; Dyes; Heavy metal ions; Oil; Water treatment
资金
- Qingdao National Laboratory for Marine Science and Technology [QNLM2016ORP0308]
- National Natural Science Foundation of China [21773219, 21878177]
- Fundamental Research Fund for the Center Universities [201861018]
- Key Development Program of Science and Technology in Shandong Province [2018GSF117041]
Because of the differences in physicochemical properties, it is of a great challenge to achieve efficient and simultaneous removal of various pollutants from water only based on one material. In this study, magnetic silica microrods (R-Fe3O4@SiO2) were successfully fabricated and used for the removal of coexisting pollutants (oil, heavy metals, soluble organic dyes) in water. R-Fe3O4@SiO2 could act as an effective solid stabilizer to disperse oil contaminants into droplets, due to its high adsorption energy at the oil water interface. The encapsulated oil by R-Fe3O4@SiO2 could be effectively separated from water by applying a magnetic field. Simultaneously, R-Fe3O4@SiO2 could adsorb soluble cationic dyes and heavy metals through electrostatic interactions. The maximal removal capacity of R-Fe3O4@SiO(2)for various pollutants in water was compared with that of some of the previously reported materials, and they showed a satisfied result. Additionally, the removal capacity of R-Fe3O4@SiO2 particles for multiple coexisting contaminants in water was evaluated. It is worthy to note that R-Fe3O4@SiO2 still showed a great removal capacity for multiple coexisting pollutants even after five runs of a sorption-desorption cycle. These results revealed that this technically simple R-Fe3O4@SiO2 material is a feasible material for the removal of various coexisting pollutants in water, and thus it holds great prospects as a candidate for the one-step water purification in practical applications.
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