期刊
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
卷 116, 期 29, 页码 14485-14494出版社
NATL ACAD SCIENCES
DOI: 10.1073/pnas.1820719116
关键词
nitrogen isotopes; fractionation; core formation; speciation; ion probe
资金
- European Research Council under the European Union [715028]
- French Government Laboratory of Excellence Initiative [ANR-10-LABX-0006]
- European Research Council (ERC) [715028] Funding Source: European Research Council (ERC)
The present-day nitrogen isotopic compositions of Earth's surficial (N-15-enriched) and deep reservoirs (N-15-depleted) differ significantly. This distribution can neither be explained by modern mantle degassing nor recycling via subduction zones. As the effect of planetary differentiation on the behavior of N isotopes is poorly understood, we experimentally determined N-isotopic fractionations during metal-silicate partitioning (analogous to planetary core formation) over a large range of oxygen fugacities (Delta IW -3.1 < logfO(2)
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