期刊
ORGANIC LETTERS
卷 21, 期 12, 页码 4469-4474出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01296
关键词
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资金
- FWO [Fund for Scientific Research-Flanders (Belgium)]
- Research Fund of the University of Leuven (KU Leuven)
- RUDN University Program 5-100
- China Scholarship Council (CSC)
- Hercules Foundation [AKUL/09/0035]
A modular and streamlined synthetic strategy for the generation of bridged indole alkaloid-like heterocycles from easily available building blocks is elaborated. This approach utilizes an Ugi four-component reaction, establishing diversity, followed by an efficient cationic gold-triggered intramolecular cascade non-oxidative dearomative spirocarbocyclization/concerted [4 + 2] cyclization cascade, furnishing these architecturally complex and distinct bridged heterocyclic scaffolds with good diastereoselectivity.
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