期刊
ORGANIC LETTERS
卷 21, 期 12, 页码 4771-4776出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01658
关键词
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资金
- National Natural Science Foundation of China [21702029]
- Thousand Plan Youth program
- Shanghai Sailing Program [17YF1400100]
- Fundamental Research Funds for the Central Universities
A regioselective, intermolecular 1,2-alkylarylation of alkenes with aryl halides and alkyl oxalates has been developed via photoredox/nickel dual catalysis. This dual-catalytic protocol involves a radical relay process, where radical addition is followed by a nickel-assisted coupling, forging two consecutive C-C bonds in a single operation. The mild and redox-neutral conditions allow for good compatibility in the scope of olefins, (hetero)aryl halides, as well as alkyl oxalates.
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