期刊
ORGANIC LETTERS
卷 21, 期 12, 页码 4525-4530出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01412
关键词
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资金
- SERB, New-Delhi [EMR/2016/006358]
- Indian Institute of Science
- R. L. Fine Chem
A weakly coordinating carboxylate directing group assisted C-H activation with maleimides leading to novel and switchable decarboxylative Heck-type and [4 + 1] annulation products catalyzed by Rh(III) has been reported. In these reactions, solvents play a vital role in switching the selectivity. An aprotic solvent, THF, leads to the decarboxylative Heck-type product while the protic solvent, TFE, results in the [4 + 1] annulation product. The methodology shows high functional group tolerance.
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