期刊
NATURE PHOTONICS
卷 13, 期 9, 页码 602-+出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41566-019-0466-7
关键词
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资金
- National Key Research and Development Program of China [2017YFA0207700]
- National Basic Research Program of China (973Program) [2015CB352003]
- Outstanding Youth Fund of Zhejiang Natural Science Foundation of China [LR18F050001]
- Natural Science Foundation of China [61804134]
- Natural Science Foundation of Fujian Province [2017J01766]
The effective detection of X-ray radiation with low threshold is essential to many medical and industrial applications. Three-dimensional (3D) organolead trihalide and double perovskites have been shown to be suitable for direct X-ray detection. However, the sensitivity and stability of 3D perovskite X-ray detectors are limited by ion motion, and there remains a demand to develop green and stable X-ray detectors with high sensitivity and low detection limit. The emerging low-dimensional perovskites have shown promising optoelectronic properties, featuring good intrinsic stability and reduced ion migration. Inspired by this, we show that our 2D layered perovskite-like (NH4)(3)Bi2I9 device provides unique anisotropic X-ray detecting performance with different crystal directions, effective suppression of ion migration and a low detection limit of 55 nGy(air) s(-1). These results will motivate new strategies to achieve a high-performance X-ray detector by utilizing 2D layered perovskite or perovskite-like materials, without requiring toxic elements.
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