期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 141, 期 31, 页码 12246-12250出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b07346
关键词
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资金
- National Institutes of Health [R01GM121678]
- School of Physical Sciences
- Chao Family Comprehensive Cancer Center at the University of California, Irvine
- Natural Sciences and Engineering Research Council of Canada [PGSD3-487506-2016]
A new catalytic radical-polar crossover annulation between two unsaturated carbonyl compounds is described. The annulation proceeds under exceptionally mild conditions and provides direct and expedient access to complex terpenoid motifs. Application of this chemistry allows for synthesis of forskolin, a densely functionalized terpenoid, in 14 steps from commercially available material.
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