期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 10, 期 14, 页码 4017-4024出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.9b01517
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- Ministry of Education, Culture, Sports, Science and Technology of the Japanese Government [25220806]
Examination of the spectral and kinetic characteristics of charge carrier recombination on nanostructured semiconductors by photoluminescence (PL) plays a significant role in understanding the photocatalytic process. Here, with an in situ single-particle PL technique, we studied the transport behavior of charge carriers in individual one-dimensional (1D) core-shell structures of CdS@CuS nanowires. Through the PL intensity changes in the single-particle PL spectroscopy, effective interfacial electron transport along the interface of CdS and CuS was observed, which contributes to the significant improvement (i.e., 13.5-fold increase) of photocatalytic H-2 production compared to that for pure CdS nanowires. The present study provides visual experimental evidence for understanding restraining of charge carrier recombination in the semiconductor.
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