期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 84, 期 16, 页码 10145-10159出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b01338
关键词
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资金
- 1000-Youth Talents Plan
- National Natural Science Foundation of China [21672097]
- National Natural Science Foundation of Jiangsu Province [BK 20170632]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
- program A for Outstanding Ph.D. candidate of Nanjing University
- Jiangsu Specially-Appointed Professor Plan
A practical single-electron-transfer-induced selective C(sp(3))-N coupling of cycloketoximes with anilines via C-C bond cleavage under copper-catalytic and synergetic photoredox/copper-catalytic reaction systems has been uncovered. These two powerful and simple protocols demonstrated excellent selectivity and good functional group compatibility without any base or ligand control. Preliminary mechanistic experiments indicated that a radical-mediated process was involved in these transformations.
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