期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 84, 期 20, 页码 12773-12783出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b01154
关键词
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资金
- JSPS [18K05114]
- Waseda University [2018K-296, 2018B-200]
- Grants-in-Aid for Scientific Research [18K05114] Funding Source: KAKEN
An efficient method for the asymmetric synthesis of 4-imidazolidinones via an iodine-catalyzed intramolecular N-H/C(sp(3))-H activation of readily available and abundant feedstocks, amino acids, and amines is described. The reaction proceeded under visible light irradiation to afford a variety of 4-imidazolidinone derivatives under mild conditions in moderate to excellent yields. Secondary and tertiary C(sp(3))-H bonds were aminated, and various functional groups were tolerated.
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