期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 361, 期 19, 页码 4442-4447出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201900550
关键词
Annulation; C-H Activation; Rhodium; Peptidomimetic; Peptide
资金
- China Scholarship Council (CSC)
- FWO [Fund for Scientific Research-Flanders (Belgium)]
- RUDN University Program 5-100
A chemoselective rhodium(III)-catalyzed cascade annulation for the construction of the indolizinone and quinolizinone scaffolds is developed. Diversification of peptidomimetics and oligopeptides is achieved in a rapid and step-economical manner through the combination of Ugi reaction and microwave-assisted rhodium(III)-catalyzed intramolecular annulation via C(sp(2))-H activation without installing a directing group.
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