期刊
SEPARATION AND PURIFICATION TECHNOLOGY
卷 212, 期 -, 页码 135-141出版社
ELSEVIER
DOI: 10.1016/j.seppur.2018.11.032
关键词
One-pot approach; Photodegradation; MoS2/CdS; Photocatalysis
资金
- National Natural Science Foundation of China [21801106]
- Shandong Province Natural Science Foundation [ZR2017PB002, ZR2018PB001]
- Research Fund for the Doctoral Program of Liaocheng University [318051640, 318051643]
Semiconductor-based photocatalytic degradation of organic pollutant shows bright prospect and has potential to address the global environmental issues. But the low efficiency, currently, is still an obstacle, which stems from ultrafast charge recombination. In this manuscript, MoS2/CdS nanodots-on-nanorods heterostructures were successfully synthesized via a novel but facile one-pot solvothermal approach with less time and energy consumption. The in-situ synthesized MoS2/CdS heterostructures with intimate interface between MoS2 and CdS facilitate photogenerated charge transportation and separation. Besides, the discrete distribution of MoS2 nanodots on CdS nanorods offers a great many active sites for organic dye degradation. As a result, the optimized MoS2/CdS hybrid shows an excellent photodegradation performance of rhodamine B (RhB) with 99.11% of RhB decomposition in 45 min, which is the advanced among all the similar catalytic systems. Our findings will give inspiration for developing low-cost and efficient catalysts for photodegradation of organic pollutants.
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