期刊
SENSORS AND ACTUATORS B-CHEMICAL
卷 284, 期 -, 页码 628-637出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2018.12.120
关键词
Electron beam irradiation; Pd nanoparticles; ZnO nanofibers; Gas sensors; H-2
资金
- Basic Science Research Program of the National Research Foundation of Korea (NRF) - Ministry of Education [2016R1D1A1B03935228]
- National Research Foundation of Korea [2016R1D1A1B03935228] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
We evaluated the hydrogen gas-sensing characteristics of Pd-loaded (0.1, 0.3, 0.6, and 1 wt%) ZnO nanofibers prepared by a facile electrospinning technique and the effect of different electron beam (e-beam) doses (50, 100, and 150 kGy) on sensing performance. The sensor loaded with 0.6 wt% Pd had the highest response to hydrogen among the Pd-loaded sensors. The sensor irradiated with 150 kGy had the high response (R-a/R-g) of 74.7-100 ppb of H-2 at 350 degrees C. Metallization effects in ZnO, the formation of structural defects due to e-beam irradiation, the catalytic activity of Pd, and the presence of ZnO-Pd heterojunctions were the main factors yielding high sensitivity towards H-2. The strategy of combining e-beam irradiation and Pd loading to enhance H-2 sensing can be applied to realize reliable gas sensors and the widespread use of hydrogen as a green energy alternative to fossil fuels.
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