期刊
ORGANIC LETTERS
卷 21, 期 9, 页码 3310-3313出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b01058
关键词
-
资金
- NSFC [21572135]
- Open Project of the State Key Laboratory of Trauma, Burn and Combined Injury, Third Military Medical University [SKLKF201601]
The alpha-regioselective asymmetric [3 + 2] annulation reaction of Morita-Baylis-Hillman carbonates from isatins and activated ortho-vinylbenzaldehyses was developed by the catalysis of a chiral tertiary amine. The sequential N-heterocyclic carbene-mediated intramolecular Stetter reaction was conducted to finally furnish the bridged 5,8-methanobenzo [7] annulen-9-one architectures incorporating a spirooxindole motif with excellent stereoselectivity.
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