期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 141, 期 23, 页码 9124-9128出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b00917
关键词
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资金
- National Key Research and Development Plan [2017YFA0505200]
- National Natural Science Foundation of China [21772110, 21822304]
The preparation of arylboronates from unactivated aryl chlorides in a transition-metal-free manner is rather challenging. There are only few examples to achieve this goal by using ultraviolet irradiation. Based on the mechanistic understanding of the diboron/methoxide/pyridine reaction system, we achieved photo activation of the in situ generated super electron donor and developed a visible-light-induced organocatalytic method for efficient borylation of unactivated aryl chlorides.
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