期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 10, 期 11, 页码 3159-3170出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.8b03721
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资金
- Australian Government through the Australian Renewable Energy Agency (ARENA)
- Australian Research Council
- Bundesministerium fur Bildung and Forschung (PRINTPERO)
- Initiating and Networking funding of the Helmholtz Association (HYIG)
- European Union's Horizon2020 program (ACTPHAST)
- Science and Technology of Nano structures research program
- Karlsruhe School of Optics & Photonics (KSOP)
- Swiss National Science Foundation via NRP70 Energy Turnaround PV2050
- Swiss National Science Foundation [176552]
- Initiating and Networking funding of the Helmholtz Association
- Initiating and Networking funding of the Helmholtz Association (Helmholtz Energy Materials Foundry (HEMF))
- Initiating and Networking funding of the Helmholtz Association (PEROSEED)
The remarkable recent progress in perovskite photovoltaics affords a novel opportunity to advance the power conversion efficiency of market-dominating crystalline silicon (c-Si) solar cells. A severe limiting factor in the development of perovskite/c-Si tandems to date has been their inferior light-harvesting ability compared to single-junction c-Si solar cells, but recent innovations have made impressive headway on this front. Here, we provide a quantitative perspective on future steps to advance perovskite/c-Si tandem photovoltaics from a light-management point of view, addressing key challenges and available strategies relevant to both the 2-terminal and 4-terminal perovskite/c-Si tandem architectures. In particular, we discuss the challenge of achieving low optical reflection in 2-terminal cells, optical shortcomings in state-of-the-art devices, the impact of transparent electrode performance, and a variety of factors which influence the optimal bandgap for perovskite top-cells. Focused attention in each of these areas will be required to make the most of the tandem opportunity.
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