期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 84, 期 9, 页码 5877-5885出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b00244
关键词
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资金
- excellence laboratory LabEx SYNORG [ANR-11-LABX-0029]
- Conseil Regional de Normandie
- European FEDER
A mild and reproducible method for the formation of a nonstabilized azomethine ylide was developed by photoinduced reaction catalyzed with eosin Y under green light irradiation. Resulting 1,3-dipole was trapped with fluoroalkenes, fluoroalkylated alkenes, and representative dipolarophiles to access pyrrolidine scaffolds, including spirocyclic compounds. The mechanism involved in this transformation was investigated, showing clearly a catalytic redox cycle with eosin Y.
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