期刊
COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING
卷 124, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.compositesa.2019.05.015
关键词
BN platelets; Functionalization; Thermal conductivity; Dielectric
资金
- National Natural Science Foundation of China [51873022]
- Support Project of High-level Teachers in Beijing Municipal Universities in the Period of 13th Five-year Plan [CITTCD201904046]
- Beijing Science and Technology Project of Beijing Municipal Education Commission [KM201710017005]
Nitrile-butadiene rubber (NBR) composites filled with functionalized BN platelets were successfully prepared to yield materials with high thermal conductivities and dielectric constants. To enhance the interfacial interactions between BN platelets and NBR matrix, non-covalent functionalization of poly(dopamine) (PDA) followed by covalent functionalization of gamma-(2,3-epoxypropoxy)propytrimethoxysilane (KH560) were employed for BN platelets surface modification to yield BN-PDA-KH560. This route led to good filler dispersion of BN-PDA-KH560 plateltes with decreased interfacial thermal resistances. Large thermal conductivity (0.409 W/mK) was achieved with 30 vol% BN-PDA-KH560/NBR composite. This value was 2.6 folds higher than that of pure NBR (0.157 W/ mK). The 30 vol% BN-PDA-KH560/NBR composite not only exhibited relatively high dielectric constant (9 at 100 Hz) but also remained low dielectric loss tangent (0.12 at 100 Hz). Overall, these findings provide a simple and effective route for preparing high-performance NBR composites with large thermal conductivities and dielectric constants for potential application in electronic devices.
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