期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 58, 期 27, 页码 9099-9103出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201903511
关键词
amino acids; directing groups; disulfides; rhodium; thiolation
资金
- National Natural Science Foundation of China [21671097, 21331002]
- Fundamental Research Funds for the Central Universities
A ligand-promoted Rh-III-catalyzed C(sp(2))-H activation/thiolation of benzamides has been developed. Using bidentate mono-N-protected amino acid ligands led to the first example of RhIII-catalyzed aryl thiolation reactions directed by weakly coordinating directing amide groups. The reaction tolerates a broad range of amides and disulfide reagents.
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