期刊
RESULTS IN PHYSICS
卷 12, 期 -, 页码 861-866出版社
ELSEVIER
DOI: 10.1016/j.rinp.2018.12.063
关键词
Colossal magnetoresistance; Double exchange mechanism; Metal-insulator temperature; Activation energy; Conduction mechanism
资金
- Research Management Centre (RMC), Universiti Teknologi MARA, Malaysia [600-IRMI/Myra 5/3/LESTARI (0150/2016)]
- Ministry of Higher Education Malaysia (MOHE), Malaysia through the Fundamental Research Grant Scheme (FRGS) [600-IRMI/FRGS 5/3(76/2016).]
The effect of yttrium (Y) substitution at La-site on structural, microstructural and electrical transport properties of (La0.7-xYx)Ca-0.3 MnO3 (x = 0.00, 0.05, 0.10, 0.15 and 0.20) were investigated. Samples were prepared by conventional solid state reaction method and structural properties of the samples were obtained using the Rietveld refinement of X-ray diffraction data. X-ray diffraction patterns show orthorhombic distorted perovskite structures. Resistivity measurement results of the LaYCaMnO3 compounds show that metal-insulator transition temperature, T-MI, shifts to lower temperature while the resistivity increases by increasing Y3+ substitution. In the metallic region (T < T-MI), experimental resistivity data were fitted to electron-electron and electron-magnon scattering mechanism while in the insulator region (T > T-MI), resistivity data were fitted to model of small polaron hopping conduction mechanism and the activation energy, E-a, increased as Y substitutions increases.
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