期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 55, 期 11, 页码 3652-3656出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201511007
关键词
biaryls; cross-coupling; homogenous catalysis; iodine; oxidation
资金
- Japan Society for the Promotion of Science (JSPS)
- Ministry of Education, Culture, Sports, Science and Technology (MEXT)
- Grants-in-Aid for Scientific Research [25860017] Funding Source: KAKEN
The direct oxidative coupling reaction has been an attractive tool for environmentally benign chemistry. Reported herein is that the hypervalent iodine catalyzed oxidative metal-free cross-coupling reaction of phenols can be achieved using Oxone as a terminal oxidant in 1,1,1,3,3,3-hexafluoropropan-2-ol (HFIP). This method features a high efficiency and regioselectivity, as well as functional-group tolerance under very mild reaction conditions without using metal catalysts.
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