期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 55, 期 10, 页码 3360-3363出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201510468
关键词
cryogenics; dysprosium; magnetocaloric effect; molecular magnetism; molecular refrigerants
资金
- Spanish MINECO [FEDER-MAT2012-38318-C03-01]
- Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]
In contrast to the mainstream research on molecular refrigerants that seeks magnetically isotropic molecules, we show that the magnetic anisotropy of dysprosium acetate tetrahydrate, [{Dy(OAc)(3)(H2O)(2)}(2)]4H(2)O (1), can be efficiently used for cooling below liquid-helium temperature. This is attained by rotating aligned single-crystal samples in a constant applied magnetic field. The envisioned advantages are fast cooling cycles and potentially compact refrigerators.
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