期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 55, 期 15, 页码 4763-4766出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201600007
关键词
alkaloids; anchimeric assistance; axinellamines; natural products; total synthesis
资金
- NIH [NIGMS R01-GM079554]
- Welch Foundation [I-1868]
- UT Southwestern
AxinellaminesA and B are broad-spectrum antibacterial pyrrole-imidazole alkaloids that have a complex polycyclic skeleton. A new asymmetric synthesis of these marine sponge metabolites is described herein, featuring an oxidative rearrangement and an anchimeric chlorination reaction.
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