期刊
SEPARATION AND PURIFICATION TECHNOLOGY
卷 210, 期 -, 页码 409-416出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.seppur.2018.08.021
关键词
DES; Ultrafiltration; Electrodialysis; Biomass
资金
- National Key Research and Development Program of China [2017YFD0601003]
- Science and Technology Planning Project of Guangdong Province, China [2017A010104005]
- Natural Science Foundation of China [21476090]
Robust membrane-based methodology with ultrafiltration and electrodialysis was employed to separate and recovery the deep eutectic solvent constituents (formed with choline chloride-ChCl and ethylene glycol-EG) after biomass fractionation using hydrothermal and DES treatment. Ultrafiltration was designed for the profound removal of lignin in DES solution. Concentration of degradation products was less than 0.1 g/L when the resulting DES solution was diluted to 40 g/L of ChCl after ultrafiltration. Electrodialysis was proven effective to separate and recovery of ChCl and EG with ChCl transferred and EG retained. Recovery ratio of ChCl and EG approached 92% and 96% and purities reached 98-99% after electrodialysis treatment. Insight gained from this study suggests a green methodology for the recovery of DES constitutes after biomass fractionation as well as the foundation for large-scale DES-based bio-refineries.
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