期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 653, 期 -, 页码 23-35出版社
ELSEVIER
DOI: 10.1016/j.scitotenv.2018.10.307
关键词
Aerosol optical depth (AOD); Air pollution; China; Topography; Land use; AOD-PM association
资金
- Natural Science Foundation of Hubei Province of China [2018CFB341]
With China's rapid economic growth, particle pollution, especially fine particulate matter (PM2.5), which is known to have adverse health impacts, has become an increasingly serious issue. Satellite aerosol optical depth (AOD), an important physical property of aerosol particles, can serve as a proxy for investigating particle pollution because it can provide observations with comprehensive spatial and temporal coverage compared with ground-level measurements. This study used an improved 14-year high-resolution AOD dataset to examine the spatial characteristics and temporal dynamics of the dominant pollutants in China from 2003 to 2016 using advanced statistical methods. The improved AOD dataset combines the Moderate Resolution Imaging Spectroradiometer (MODIS) 3-km dark target AOD and 10-km deep blue AOD datasets, which enables a comparison of aerosol loading between eastern and western China. Pixel-based analysis indicates a significant difference between eastern and western China: high AOD values were generally observed in the east with a notable decrease, while low aerosol loadings were found in western China with no distinct change. The most particle polluted areas were the North China Plain, Hubei-Hunan region, Sichuan Basin, and Guangxi-Guangdong region in eastern China and western Qinghai and Tarim Basin in western China, with changes in the national AOD average center shifting to the northwest from 2013 to 2016. The impact factor analysis based on geographically weighted regression indicates that the effect of topography on the spatial characteristics of AOD is negative and more important in eastern China, which has low elevations. Built-up areas significantly exacerbate air pollution in the areas between eastern and western China, and there is no apparent AOD-vegetation relation dominates the country. This study thus provides a comprehensive understanding of the spatiotemporal variations of particle concentrations and can facilitate environmental management, policies to alleviate particle pollution, and health risk assessment studies. (c) 2018 Elsevier B.V. All rights reserved.
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