期刊
SCIENCE CHINA-CHEMISTRY
卷 62, 期 4, 页码 500-505出版社
SCIENCE PRESS
DOI: 10.1007/s11426-018-9426-2
关键词
drop-coating; PEDOT:PSS; flexible electrodes; figure of merit; organic solar cells
资金
- National Key R&D Program of China [2017YFE0106000]
- National Natural Science Foundation of China [51773212, 21574144, 21674123, 61705240]
- Zhejiang Provincial Natural Science Foundation of China [LR16B040002]
- Ningbo Municipal Science and Technology Innovative Research Team [2015B11002, 2016B10005]
- CAS Interdisciplinary Innovation Team
- CAS Key Project of Frontier Science Research [QYZDBSSW-SYS030]
- CAS Key Project of International Cooperation [174433KYSB20160065]
Highly conductive poly(3,4-ethylenedioxythiophene):poly(styrene-sulfonic acid) (PEDOT:PSS) has been explored to fabricate flexible and stretchable conductors. Generally, PEDOT:PSS transparent anodes are prepared by spin-coating method. In this article, we adopt a method by dropping PEDOT:PSS aqueous solution on the PET plastic substrate to fabricate flexible electrodes. Compared with spin coating, drop-coating is simple and cost-effective with large-area fabrications. Through this method, we fabricated highly transparent conductive electrodes and systematically studied their electrical, optical, morphological and mechanical properties. With dimethyl sulfoxide/methanesulfonic acid (DMSO/MSA) treated PEDOT:PSS electrode, bendable devices based on non-fullerene system displayed an open-circuit voltage of 0.925 V, a fill factor of 70.74%, and a high power conversion efficiency (PCE) of 10.23% under 100 mW cm(-2) illumination, which retained over 80% of the initial PCE value after 1000 bending cycles. Based on the findings, drop-coated PEDOT:PSS electrodes exhibited high suitability for the development of large-area and high-efficiency printed solar cell modules in the future.
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