4.7 Review

Aerosol Mixing State: Measurements, Modeling, and Impacts

期刊

REVIEWS OF GEOPHYSICS
卷 57, 期 2, 页码 187-249

出版社

AMER GEOPHYSICAL UNION
DOI: 10.1029/2018RG000615

关键词

aerosol mixing state; aerosol climate impacts; aerosol modeling; aerosol measurements

资金

  1. DOE [DE-SC0019192]
  2. NSF [CHE-1654149, AGS-1703019, AGS-1254428, CMMI-1150490]
  3. Sloan Research Fellowship in Chemistry
  4. Susan Lipschutz Fellowship Award from the University of Michigan Rackham Graduate School
  5. U.S. Department of Energy (DOE) [DE-SC0019192] Funding Source: U.S. Department of Energy (DOE)

向作者/读者索取更多资源

Atmospheric aerosols are complex mixtures of different chemical species, and individual particles exist in many different shapes and morphologies. Together, these characteristics contribute to the aerosol mixing state. This review provides an overview of measurement techniques to probe aerosol mixing state, discusses how aerosol mixing state is represented in atmospheric models at different scales, and synthesizes our knowledge of aerosol mixing state's impact on climate-relevant properties, such as cloud condensation and ice nucleating particle concentrations, and aerosol optical properties. We present these findings within a framework that defines aerosol mixing state along with appropriate mixing state metrics to quantify it. Future research directions are identified, with a focus on the need for integrating mixing state measurements and modeling.

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