期刊
ORGANIC LETTERS
卷 21, 期 6, 页码 1559-1563出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b03927
关键词
-
资金
- National Natural Science Foundation of China [21772077, 21372108]
Iron-catalyzed intramolecular C-H amination of aliphatic azides has recently emerged as a powerful tool for the preparation of nitrogen heterocycles. This paper reports that alpha-azidyl amides can be converted in high efficacy to imidazolinone compounds via intramolecular C(sp(3))-H amination by the action of a simple catalytic system composed of FeCl2 and a beta-diketiminate ligand. The reactions provide a simple and atom-economical approach toward polysubstituted imidazolinones.
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