期刊
ORGANIC LETTERS
卷 21, 期 5, 页码 1434-1437出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b00187
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资金
- University of Basel
1,n-Metal shift is an elegant alternative approach enabling the functionalization of remote C H bonds from simple precursors. In this work, we report a novel and simple Pd-0-catalyzed domino reaction involving 1,4-palladium shift and C(sp(3))-H activation and leading to (fused) five-membered rings. This method allowed access to a broad range of valuable arylidene gamma-lactams and indanones and was applied to the formal synthesis of (-)-pyrrolam.
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