期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 141, 期 12, 页码 4820-4823出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.9b01739
关键词
-
资金
- Chemistry Department for the Windt Graduate Fellowship
Described is a concise total synthesis of (-)-ambiguine P, a cycloheptane-containing member of the hapalindole alkaloids. The challenging pentacyclic framework of the natural product was assembled rapidly via a [4 + 3] cycloaddition reaction-inspired strategy, and the tertiary hydroxy group was introduced by an NBS-mediated bromination-nucleophilic substitution sequence.
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