期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 84, 期 5, 页码 2870-2878出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b00010
关键词
-
资金
- National Natural Science Foundation of China [21320102002, 91427301]
Pd(OAc)(2)-catalyzed intramolecular dehydrogenative cross-coupling reaction between tertiary enamides, which were derived from the condensation of 2-arylethylamines and methyl o-acetylbenzoate, and arenes enabled synthesis of 7,8-dihydro-5H-benzo[4,5]azepino[2,1-a]-isoindol-5-one derivatives under mild conditions. The synthetic method was applied in the total synthesis of aporhoeadane alkaloids palmanine, lennoxamine, and chilenamine in only three or four steps.
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