期刊
JOURNAL OF APPLIED PHYSICS
卷 125, 期 7, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.5064371
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资金
- U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02-07ER46386]
ZnS1-xOx is a highly mismatched semiconductor alloy with potential light-emitting and solar-cell applications. In this work, optical transmission spectroscopy and a modified derivative method were employed to determine the room-temperature bandgap of cubic (zinc blende) ZnS1-xOx from x = 0.01 to 0.3. The bandgap drops steeply for dilute oxygen concentrations, followed by a more gradual decrease for x > 0.05. This nonlinear behavior is attributed to a transition from isolated oxygen impurities to pairs and larger clusters. Alloying with x = 0.3 causes bandgap to drop from 3.7 to 3.1 eV. Previous work showed that the bandgap of wurtzite ZnS1-xOx shifts from 3.7 to 2.8 eV over the same composition range. Published under license by AIP Publishing.
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