期刊
CHEMICAL REVIEWS
卷 119, 期 6, 页码 3962-4179出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemrev.8b00400
关键词
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资金
- National Natural Science Foundation of China [51672089, 20906034]
- Science and Technology Planning Project of Guangdong Province [2015B020215011]
- State Key Laboratory of Advanced Technology for Material Synthesis and Processing (Wuhan University of Technology) [2015-KF-7]
- NSFC [51320105001, U1705251, 21433007]
- 973 program [2013CB632402]
- Natural Science Foundation of Hubei Province [2015CFA001]
- Innovative Research Funds of SKLWUT [2017-ZD-4]
- U.S. National Science Foundation [DMR-1609061]
- College of Arts and Sciences, University of Missouri-Kansas City
Photoreduction of CO2 into sustainable and green solar fuels is generally believed to be an appealing solution to simultaneously overcome both environmental problems and energy crisis. The low selectivity of challenging multi-electron CO2 photoreduction reactions makes it one of the holy grails in heterogeneous photocatalysis. This Review highlights the important roles of cocatalysts in selective photocatalytic CO2 reduction into solar fuels using semiconductor catalysts. A special emphasis in this review is placed on the key role, design considerations and modification strategies of cocatalysts for CO2 photoreduction. Various cocatalysts, such as the biomimetic, metal-based, metal-free, and multifunctional ones, and their selectivity for CO2 photoreduction are summarized and discussed, along with the recent advances in this area. This Review provides useful information for the design of highly selective cocatalysts for photo(electro)reduction and electroreduction of CO2 and complements the existing reviews on various semiconductor photocatalysts.
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