期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 58, 期 30, 页码 10061-10073出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201901361
关键词
charge separation; oxidation; photocatalysis; semiconductors; surface chemistry
资金
- National Natural Science Foundations of China [51672258]
- Australian Research Council (ARC) [DE150101306, LP160100927]
- Australian Research Council [DE150101306] Funding Source: Australian Research Council
Semiconductor photocatalysis as a desirable technology shows great potential in environmental remediation and renewable energy generation, but its efficiency is severely restricted by the rapid recombination of charge carriers in the bulk phase and on the surface of photocatalysts. Polarization has emerged as one of the most effective strategies for addressing the above-mentioned issues, thus effectively promoting photocatalysis. This review summarizes the recent advances on improvements of photocatalytic activity by polarization-promoted bulk and surface charge separation. Highlighted is the recent progress in charge separation advanced by different types of polarization, such as macroscopic polarization, piezoelectric polarization, ferroelectric polarization, and surface polarization, and the related mechanisms. Finally, the strategies and challenges for polarization enhancement to further enhance charge separation and photocatalysis are discussed.
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