期刊
ADVANCED FUNCTIONAL MATERIALS
卷 29, 期 16, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201900265
关键词
combustion synthesize; electron-transporting layer; intrinsic passivation; perovskite solar cell; zinc oxide
类别
资金
- Northwestern University LEAP Center, US Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]
- Northwestern UniversityMRSEC [NSFDMR-1720139]
- Flexterra Corp.
- MRSEC program [NSFDMR-1720139]
- International Institute for Nanotechnology (IIN)
- Keck Foundation
- State of Illinois
- Shenzhen Peacock Plan project [KQTD20140630110339343]
- National Key R&D Program of China [2018YFB0407100-02]
- Foundation for Innovation Research Groups of the National Natural Science Foundation of China (NSFC) [61421002]
- Foundation of NSFC [61675041, 51703019]
- China Scholarship Council [201706070042]
Perovskite solar cells (PSCs) have advanced rapidly with power conversion efficiencies (PCEs) now exceeding 22%. Due to the long diffusion lengths of charge carriers in the photoactive layer, a PSC device architecture comprising an electron-transporting layer (ETL) is essential to optimize charge flow and collection for maximum performance. Here, a novel approach is reported to low temperature, solution-processed ZnO ETLs for PSCs using combustion synthesis. Due to the intrinsic passivation effects, high crystallinity, matched energy levels, ideal surface topography, and good chemical compatibility with the perovskite layer, this combustion-derived ZnO enables PCEs approaching 17-20% for three types of perovskite materials systems with no need for ETL doping or surface functionalization.
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