4.8 Article

Nitrogen-Doped Porous Carbon Nanosheets Templated from g-C3N4 as Metal-Free Electrocatalysts for Efficient Oxygen Reduction Reaction

期刊

ADVANCED MATERIALS
卷 28, 期 25, 页码 5080-5086

出版社

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201600398

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资金

  1. Ministry of Science and Technology of China [2014CB239402, 2013CB834505]
  2. Chinese Academy of Science [KGZD-EW-T05]
  3. National Natural Science Foundation of China [51322213, 21401206, 21401207, 51172245, 51571170, 21301183]
  4. Beijing Natural Science Foundation [2152033, 2154058]
  5. National Program for Support of Top-notch Young Professional

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Nitrogen-doped porous carbon nano-sheets (N-CNS) are synthesized by hydro thermal carbon coating of g-C3N4 nanosheets followed by high-temperature treatment in N-2. g-C3N4 serves as a template, nitrogen source, and porogen in the synthesis. This approach yields N-CNS with a high nitrogen content and comparable oxygen reduction reaction catalytic activities to commercial Pt/C catalysts in alkaline media.

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